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Optical properties of light absorbing carbon aggregates mixed with sulfate: assessment of different model geometries for climate forcing calculations
SMHI, Research Department, Air quality.ORCID iD: 0000-0001-5695-1356
2012 (English)In: Optics Express, ISSN 1094-4087, E-ISSN 1094-4087, Vol. 20, no 9Article in journal (Refereed) Published
Abstract [en]

Light scattering by light absorbing carbon (LAC) aggregates encapsulated into sulfate shells is computed by use of the discrete dipole method. Computations are performed for a UV, visible, and IR wavelength, different particle sizes, and volume fractions. Reference computations are compared to three classes of simplified model particles that have been proposed for climate modeling purposes. Neither model matches the reference results sufficiently well. Remarkably, more realistic core-shell geometries fall behind homogeneous mixture models. An extended model based on a core-shell-shell geometry is proposed and tested. Good agreement is found for total optical cross sections and the asymmetry parameter. (C) 2012 Optical Society of America

Place, publisher, year, edition, pages
2012. Vol. 20, no 9
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Environmental Sciences
Research subject
Environment
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URN: urn:nbn:se:smhi:diva-462DOI: 10.1364/OE.20.010042ISI: 000303989300074PubMedID: 22535095OAI: oai:DiVA.org:smhi-462DiVA: diva2:806253
Available from: 2015-04-20 Created: 2015-04-14 Last updated: 2017-12-04Bibliographically approved

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Kahnert, Michael

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